疫情防控期间新疆背景站大气黑碳浓度的变化

Variations in Atmospheric Black Carbon at a Xinjiang Background Site During the COVID-19 Lockdown

  • 摘要: 人为活动和野火排放的黑碳(blackcarbon,BC)对太阳辐射具有较强的吸收作用,是气候环境变化的敏感因子.在人口稀少的偏远乡镇,对人为活动的管控是否能显著改变大气中BC含量,进而改善大气环境,目前鲜有研究.本文基于我国西北边境吉木乃县的BC观测数据,选取防控期与非防控两种典型时段,分析比较了不同人为活动强度下当地BC浓度的变化特征.结果表明:在防控期间,吉木乃县背景站观测到的BC浓度由0.47 µg·m−3显著下降至0.23 µg·m−3,降幅达到51%.模型分析结果表明,BC在防控前、中和后期的浓度与气象归一化后的浓度变化基本一致,表明防控期内气象条件对该区域大气BC浓度影响较小,其变化主要受人为排放影响.基于风场观测数据的分析表明,防控期间BC浓度的变化主要受观测站上风向吉木乃县区域人为排放的影响.本研究同时发现,尽管实施了防控措施,2019-2020年秋冬季的BC浓度仍高于2023-2024年秋冬季.浓度权重轨迹分析进一步显示,在2019-2020年秋冬季,长距离传输的主要区域来源位于观测点正西方向;而在2023-2024年秋冬季,该来源区域则转移至西北方向.上风向BC源区的空间差异可能是导致这两个年份观测结果不同的原因.

     

    Abstract: Black carbon (BC), emitted from anthropogenic activities and wildfires, strongly absorbs solar radiation and is recognized as a sensitive indicator of climate and environmental change. In sparsely populated remote areas, however, whether restrictions on human activities can significantly alter ambient BC concentrations and thereby improve air quality remains poorly understood. Based on BC observations at a background site in Jimunai County, located in the northwestern border region of China, this study selected two representative periods (lockdown and non-lockdown periods) to investigate the variations in carbonaceous aerosols under different levels of anthropogenic activity. The results show that during the lockdown period, the BC concentration at the Jimunai background site decreased significantly from 0.47 µg·m−3 to 0.23 µg·m−3, representing a reduction of 51%. Model analysis indicates that the variations in observed BC concentrations before, during, and after the lockdown are generally consistent with meteorologically normalized concentrations, suggesting that meteorological conditions had a limited influence on BC levels during the lockdown, and that the observed changes were mainly driven by variations in anthropogenic emissions. Analysis of wind field observations further reveals that BC variations during the lockdown were primarily influenced by anthropogenic emissions from the upwind Jimunai region. In addition, despite the implementation of lockdown measures, BC concentrations in the autumn–winter period of 2019-2020 remained higher than 2023-2024. Concentration-weighted trajectory (CWT) analysis further shows that the dominant source regions of long-range transport were located to the west of the observation site in 2019-2020, but shifted to the northwest in 2023-2024. The spatial differences in upwind BC source regions may account for the discrepancies between the two periods.

     

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